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RAS PresidiumДоклады Российской академии наук. Химия, науки о материалах Doklady Chemistry

  • ISSN (Print) 2686-9535
  • ISSN (Online) 3034-5111

STRUCTURAL DIVERSITY AND LUMINESCENT PROPERTIES OF LANTHANIDE COORDINATION POLYMERS WITH 4,7-DI(4-CARBOXYPYRAZOLE-1-YL)-2,1,3-BENZOXADIAZOLE

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PII
S30345111S2686953525030014-1
DOI
10.7868/S3034511125030014
Publication type
Article
Status
Published
Authors
E.R. Dudko
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
D.I. Pavlov
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
A.A. Ryadun
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
Yu.A. Kenzhebayeva
  • Affiliation: ITMO University
D.G. Samsonenko
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
V.A. Milichko
  • Affiliation: ITMO University
V.P. Fedin
  • Occupation: Academician of the RAS
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
A.S. Potapov
  • Affiliation: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences
Volume/ Edition
Volume 522 / Issue number 1
Pages
3-13
Abstract
A series of new lanthanide metal-organic coordination polymers with 4,7-di(4-carboxypyrazol-1-yl)-2,1,3-benzoxadiazole were synthesized. It was established that, depending on the position of element in the lanthanide series, products of four structural types are formed. In the case of the Ce cation, the coordination polymer represents 1D chains, for Pr–Er cations it is a 2D layered structure with layer concatenation, and for the late lanthanides Tm–Lu two types of layered coordination polymers were identified, differing in the carboxylate group coordination mode and the number of coordinated water molecules in the coordination sphere of the central ion. The coordination polymers of Sm, Eu, Gd, and Tb exhibit only ligand-centered luminescence with a maximum in the range of 540–550 nm, while the luminescence spectrum of Nd coordination polymer additionally contains characteristic bands of metal-centered emission in the near infrared range at 878, 1054, 1330, and 1568 nm.
Keywords
лантаноиды 2,1,3-бензохалькогенадиазолы 2,1,3-бензоксадиазол люминесценция пиразол металл-органические координационные полимеры
Date of publication
01.06.2025
Year of publication
2025
Number of purchasers
0
Views
20

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